Bhattacharyya, Sarika and Bagchi, Biman (1997) Bimodality in the dynamic response of a supercooled liquid. In: Journal of Chemical Physics, 106 (17). pp. 7262-7267.
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In order to understand the emergence and the influence of the ''cage effect'' in the dynamic response of a liquid, a detailed theoretical study of the frequency dependent friction of a Lennard-Jones liquid is carried out by using the mode coupling theory. The frequency dependent friction becomes increasingly bimodal in nature as the density of the liquid is increased beyond the liquid-solid coexistence line. The bimodality is most clearly manifested in the frequency dependence of the imaginary part of the friction. The mode coupling theory provides a nice physical interpretation of these results which are also in good agreement with the existing computer simulations.
|Item Type:||Journal Article|
|Additional Information:||Copyright of this article belongs to American institute of Physics.|
|Department/Centre:||Division of Chemical Sciences > Solid State & Structural Chemistry Unit|
|Date Deposited:||09 Mar 2009 05:40|
|Last Modified:||19 Sep 2010 05:02|
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